
Hierarchically Au-functionalized derived ultrathin NiO nanosheets for highly sensitive electrochemical hydrazine detection
- Author
- Wenda Wang, Zhenting Zhao, Qian Lei, Wenlei Zhang, Pengwei Li, Wendong Zhang, Serge Zhuiykov (UGent) and Jie Hu
- Organization
- Abstract
- A highly sensitive hierarchical electrochemical sensing nanostructures have been successfully synthesized by hydrothermal and chemical deposition methods using Au nanoparticles (AuNPs)-functionalized Metal-organic frameworks (MOF) derived oxide nickel nanosheets (NiO NSs) on nickel foam (AuNPs@NiO NSs/NF). The morphological characterization of AuNPs@NiO NSs/NF nanomaterials was investigated by scanning electron microscope (SEM), energy dispersive X-ray spectrometry (EDS) and X-ray diffraction (XRD) techniques. The electrochemical behaviors of AuNPs@NiO NSs/NF sensors were evaluated by cyclic voltammetry (CV), electrochemical impedance spectroscopy (EIS) and amperometric response (i-t). The measured results of AuNPs@NiO NSs/NF sensor shows good electrochemical properties, including high sensitivity of 17.80 mu A.mu M-1.cm(-2), wide linear range from 0.2 to 300 mu M, a low detection limit (LOD) (S/N = 3) of 0.04 mu M, limit of quantification (LOQ) of 0.13 mu M and as well as great selectivity and long-time stability. Moreover, the electrochemical sensor has also been demonstrated excellent hydrazine properties in the real environmental samples. The excellent electrochemical performance of AuNPs@NiO NSs/NF sensor can be attributed to the hierarchical nanostructure of nickel-metal frameworks and synergistic catalysis effect of Au nanoparticles, which is promising as highly sensitive material for electrochemical sensor applications.
- Keywords
- Surfaces, Coatings and Films, Metal-organic frameworks, NiO nanosheets, Au nanoparticles, Hydrothermal, Hydrazine sensor, REDUCED GRAPHENE OXIDE, ELECTROCATALYTIC OXIDATION, AMPEROMETRIC SENSOR, GOLD NANOPARTICLES, CARBON NANOTUBES, CHEMICAL SENSOR, ELECTRODE, ZNO, FABRICATION, PLATFORM
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Citation
Please use this url to cite or link to this publication: http://hdl.handle.net/1854/LU-8686552
- MLA
- Wang, Wenda, et al. “Hierarchically Au-Functionalized Derived Ultrathin NiO Nanosheets for Highly Sensitive Electrochemical Hydrazine Detection.” APPLIED SURFACE SCIENCE, vol. 542, 2021, doi:10.1016/j.apsusc.2020.148539.
- APA
- Wang, W., Zhao, Z., Lei, Q., Zhang, W., Li, P., Zhang, W., … Hu, J. (2021). Hierarchically Au-functionalized derived ultrathin NiO nanosheets for highly sensitive electrochemical hydrazine detection. APPLIED SURFACE SCIENCE, 542. https://doi.org/10.1016/j.apsusc.2020.148539
- Chicago author-date
- Wang, Wenda, Zhenting Zhao, Qian Lei, Wenlei Zhang, Pengwei Li, Wendong Zhang, Serge Zhuiykov, and Jie Hu. 2021. “Hierarchically Au-Functionalized Derived Ultrathin NiO Nanosheets for Highly Sensitive Electrochemical Hydrazine Detection.” APPLIED SURFACE SCIENCE 542. https://doi.org/10.1016/j.apsusc.2020.148539.
- Chicago author-date (all authors)
- Wang, Wenda, Zhenting Zhao, Qian Lei, Wenlei Zhang, Pengwei Li, Wendong Zhang, Serge Zhuiykov, and Jie Hu. 2021. “Hierarchically Au-Functionalized Derived Ultrathin NiO Nanosheets for Highly Sensitive Electrochemical Hydrazine Detection.” APPLIED SURFACE SCIENCE 542. doi:10.1016/j.apsusc.2020.148539.
- Vancouver
- 1.Wang W, Zhao Z, Lei Q, Zhang W, Li P, Zhang W, et al. Hierarchically Au-functionalized derived ultrathin NiO nanosheets for highly sensitive electrochemical hydrazine detection. APPLIED SURFACE SCIENCE. 2021;542.
- IEEE
- [1]W. Wang et al., “Hierarchically Au-functionalized derived ultrathin NiO nanosheets for highly sensitive electrochemical hydrazine detection,” APPLIED SURFACE SCIENCE, vol. 542, 2021.
@article{8686552, abstract = {{A highly sensitive hierarchical electrochemical sensing nanostructures have been successfully synthesized by hydrothermal and chemical deposition methods using Au nanoparticles (AuNPs)-functionalized Metal-organic frameworks (MOF) derived oxide nickel nanosheets (NiO NSs) on nickel foam (AuNPs@NiO NSs/NF). The morphological characterization of AuNPs@NiO NSs/NF nanomaterials was investigated by scanning electron microscope (SEM), energy dispersive X-ray spectrometry (EDS) and X-ray diffraction (XRD) techniques. The electrochemical behaviors of AuNPs@NiO NSs/NF sensors were evaluated by cyclic voltammetry (CV), electrochemical impedance spectroscopy (EIS) and amperometric response (i-t). The measured results of AuNPs@NiO NSs/NF sensor shows good electrochemical properties, including high sensitivity of 17.80 mu A.mu M-1.cm(-2), wide linear range from 0.2 to 300 mu M, a low detection limit (LOD) (S/N = 3) of 0.04 mu M, limit of quantification (LOQ) of 0.13 mu M and as well as great selectivity and long-time stability. Moreover, the electrochemical sensor has also been demonstrated excellent hydrazine properties in the real environmental samples. The excellent electrochemical performance of AuNPs@NiO NSs/NF sensor can be attributed to the hierarchical nanostructure of nickel-metal frameworks and synergistic catalysis effect of Au nanoparticles, which is promising as highly sensitive material for electrochemical sensor applications.}}, articleno = {{148539}}, author = {{Wang, Wenda and Zhao, Zhenting and Lei, Qian and Zhang, Wenlei and Li, Pengwei and Zhang, Wendong and Zhuiykov, Serge and Hu, Jie}}, issn = {{0169-4332}}, journal = {{APPLIED SURFACE SCIENCE}}, keywords = {{Surfaces,Coatings and Films,Metal-organic frameworks,NiO nanosheets,Au nanoparticles,Hydrothermal,Hydrazine sensor,REDUCED GRAPHENE OXIDE,ELECTROCATALYTIC OXIDATION,AMPEROMETRIC SENSOR,GOLD NANOPARTICLES,CARBON NANOTUBES,CHEMICAL SENSOR,ELECTRODE,ZNO,FABRICATION,PLATFORM}}, language = {{eng}}, pages = {{10}}, title = {{Hierarchically Au-functionalized derived ultrathin NiO nanosheets for highly sensitive electrochemical hydrazine detection}}, url = {{http://doi.org/10.1016/j.apsusc.2020.148539}}, volume = {{542}}, year = {{2021}}, }
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