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Two-dimensional material interface engineering for efficient perovskite large-area modules

(2019) ACS ENERGY LETTERS. 4(8). p.1862-1871
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Abstract
In this work, we demonstrate the successful application of two-dimensional (2D) materials, i.e., graphene and functionalized MoS2, in perovskite solar cells (PSCs) by interface engineering the standard mesoscopic n-i-p structure. The use of 2D materials has the dual role to improve both the stability and the overall power conversion efficiency (PCE) of the PSCs compared to standard devices. The application of 2D materials is successfully extended to large-area perovskite solar modules (PSMs), achieving PCEs of 13.4% and 15.3% on active areas of 108 cm(2) and 82 cm(2), respectively. This performance results in record-high active area-indexed aperture PCE (AIAPCE) of 1266.5% cm(2). In addition, the 2D materials-based PSMs show a stability under a prolonged (>1000 h) thermal stress test at 65 degrees C (ISOS-D2), representing a crucial advancement in the exploitation of perovskite photovoltaic technology.
Keywords
HOLE-TRANSPORT LAYER, SOLAR-CELLS, HIGHLY EFFICIENT, SPIRO-OMETAD, INDUCED DEGRADATION, LOW-TEMPERATURE, GRAPHENE OXIDE, THIN-FILMS, STABILITY, CHALLENGES

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MLA
Agresti, Antonio, et al. “Two-Dimensional Material Interface Engineering for Efficient Perovskite Large-Area Modules.” ACS ENERGY LETTERS, vol. 4, no. 8, 2019, pp. 1862–71.
APA
Agresti, A., Pescetelli, S., Palma, A. L., Martín-García, B., Najafi, L., Bellani, S., … Di Carlo, A. (2019). Two-dimensional material interface engineering for efficient perovskite large-area modules. ACS ENERGY LETTERS, 4(8), 1862–1871.
Chicago author-date
Agresti, Antonio, Sara Pescetelli, Alessandro Lorenzo Palma, Beatriz Martín-García, Leyla Najafi, Sebastiano Bellani, Iwan Moreels, Mirko Prato, Francesco Bonaccorso, and Aldo Di Carlo. 2019. “Two-Dimensional Material Interface Engineering for Efficient Perovskite Large-Area Modules.” ACS ENERGY LETTERS 4 (8): 1862–71.
Chicago author-date (all authors)
Agresti, Antonio, Sara Pescetelli, Alessandro Lorenzo Palma, Beatriz Martín-García, Leyla Najafi, Sebastiano Bellani, Iwan Moreels, Mirko Prato, Francesco Bonaccorso, and Aldo Di Carlo. 2019. “Two-Dimensional Material Interface Engineering for Efficient Perovskite Large-Area Modules.” ACS ENERGY LETTERS 4 (8): 1862–1871.
Vancouver
1.
Agresti A, Pescetelli S, Palma AL, Martín-García B, Najafi L, Bellani S, et al. Two-dimensional material interface engineering for efficient perovskite large-area modules. ACS ENERGY LETTERS. 2019;4(8):1862–71.
IEEE
[1]
A. Agresti et al., “Two-dimensional material interface engineering for efficient perovskite large-area modules,” ACS ENERGY LETTERS, vol. 4, no. 8, pp. 1862–1871, 2019.
@article{8642422,
  abstract     = {In this work, we demonstrate the successful application of two-dimensional (2D) materials, i.e., graphene and functionalized MoS2, in perovskite solar cells (PSCs) by interface engineering the standard mesoscopic n-i-p structure. The use of 2D materials has the dual role to improve both the stability and the overall power conversion efficiency (PCE) of the PSCs compared to standard devices. The application of 2D materials is successfully extended to large-area perovskite solar modules (PSMs), achieving PCEs of 13.4% and 15.3% on active areas of 108 cm(2) and 82 cm(2), respectively. This performance results in record-high active area-indexed aperture PCE (AIAPCE) of 1266.5% cm(2). In addition, the 2D materials-based PSMs show a stability under a prolonged (>1000 h) thermal stress test at 65 degrees C (ISOS-D2), representing a crucial advancement in the exploitation of perovskite photovoltaic technology.},
  author       = {Agresti, Antonio and Pescetelli, Sara and Palma, Alessandro Lorenzo and Martín-García, Beatriz and Najafi, Leyla and Bellani, Sebastiano and Moreels, Iwan and Prato, Mirko and Bonaccorso, Francesco and Di Carlo, Aldo},
  issn         = {2380-8195},
  journal      = {ACS ENERGY LETTERS},
  keywords     = {HOLE-TRANSPORT LAYER,SOLAR-CELLS,HIGHLY EFFICIENT,SPIRO-OMETAD,INDUCED DEGRADATION,LOW-TEMPERATURE,GRAPHENE OXIDE,THIN-FILMS,STABILITY,CHALLENGES},
  language     = {eng},
  number       = {8},
  pages        = {1862--1871},
  title        = {Two-dimensional material interface engineering for efficient perovskite large-area modules},
  url          = {http://dx.doi.org/10.1021/acsenergylett.9b01151},
  volume       = {4},
  year         = {2019},
}

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