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One-pot synthesis of Pt catalysts based on layered double hydroxides: an application in propane dehydrogenation

Matthias Filez UGent, Evgeniy Redekop, Hilde Poelman UGent, Vladimir Galvita UGent, M Meledina, S Turner, G Van Tendeloo, Christophe Detavernier UGent and Guy Marin UGent (2016) CATALYSIS SCIENCE & TECHNOLOGY. 2016(6). p.1863-1869
abstract
Simple methods for producing noble metal catalysts with well-defined active sites and improved performance are highly desired in the chemical industry. However, the development of such methods still presents a formidable synthetic challenge. Here, we demonstrate a one-pot synthesis route for the controlled production of bimetallic Pt-In catalysts based on the single-step formation of Mg,Al,Pt,In-containing layered double hydroxides (LDHs). Besides their simple synthesis, these Pt-In catalysts exhibit superior propane dehydrogenation activity compared to their multi-step synthesized analogs. The presented material serves as a showcase for the one-pot synthesis of a broader class of LDH-derived mono- and multimetallic Pt catalysts. The compositional flexibility provided by LDH materials can pave the way towards high-performing Pt-based catalysts with tunable physicochemical properties.
Please use this url to cite or link to this publication:
author
organization
year
type
journalArticle (original)
publication status
published
subject
journal title
CATALYSIS SCIENCE & TECHNOLOGY
volume
2016
issue
6
pages
1863 - 1869
Web of Science type
Article
Web of Science id
000372172800031
JCR category
CHEMISTRY, PHYSICAL
JCR impact factor
5.773 (2016)
JCR rank
27/145 (2016)
JCR quartile
1 (2016)
ISSN
2044-4753
DOI
10.1039/C5CY01274K
language
English
UGent publication?
yes
classification
A1
copyright statement
I have transferred the copyright for this publication to the publisher
id
8054497
handle
http://hdl.handle.net/1854/LU-8054497
date created
2016-08-25 10:40:02
date last changed
2017-03-09 12:54:26
@article{8054497,
  abstract     = {Simple methods for producing noble metal catalysts with well-defined active sites and improved performance are highly desired in the chemical industry. However, the development of such methods still presents a formidable synthetic challenge. Here, we demonstrate a one-pot synthesis route for the controlled production of bimetallic Pt-In catalysts based on the single-step formation of Mg,Al,Pt,In-containing layered double hydroxides (LDHs). Besides their simple synthesis, these Pt-In catalysts exhibit superior propane dehydrogenation activity compared to their multi-step synthesized analogs. The presented material serves as a showcase for the one-pot synthesis of a broader class of LDH-derived mono- and multimetallic Pt catalysts. The compositional flexibility provided by LDH materials can pave the way towards high-performing Pt-based catalysts with tunable physicochemical properties.},
  author       = {Filez, Matthias and Redekop, Evgeniy and Poelman, Hilde and Galvita, Vladimir and Meledina, M and Turner, S and Van Tendeloo, G and Detavernier, Christophe and Marin, Guy},
  issn         = {2044-4753},
  journal      = {CATALYSIS SCIENCE \& TECHNOLOGY},
  language     = {eng},
  number       = {6},
  pages        = {1863--1869},
  title        = {One-pot synthesis of Pt catalysts based on layered double hydroxides: an application in propane dehydrogenation},
  url          = {http://dx.doi.org/10.1039/C5CY01274K},
  volume       = {2016},
  year         = {2016},
}

Chicago
Filez, Matthias, Evgeniy Redekop, Hilde Poelman, Vladimir Galvita, M Meledina, S Turner, G Van Tendeloo, Christophe Detavernier, and Guy Marin. 2016. “One-pot Synthesis of Pt Catalysts Based on Layered Double Hydroxides: An Application in Propane Dehydrogenation.” Catalysis Science & Technology 2016 (6): 1863–1869.
APA
Filez, M., Redekop, E., Poelman, H., Galvita, V., Meledina, M., Turner, S., Van Tendeloo, G., et al. (2016). One-pot synthesis of Pt catalysts based on layered double hydroxides: an application in propane dehydrogenation. CATALYSIS SCIENCE & TECHNOLOGY, 2016(6), 1863–1869.
Vancouver
1.
Filez M, Redekop E, Poelman H, Galvita V, Meledina M, Turner S, et al. One-pot synthesis of Pt catalysts based on layered double hydroxides: an application in propane dehydrogenation. CATALYSIS SCIENCE & TECHNOLOGY. 2016;2016(6):1863–9.
MLA
Filez, Matthias, Evgeniy Redekop, Hilde Poelman, et al. “One-pot Synthesis of Pt Catalysts Based on Layered Double Hydroxides: An Application in Propane Dehydrogenation.” CATALYSIS SCIENCE & TECHNOLOGY 2016.6 (2016): 1863–1869. Print.