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Use of compound-specific nitrogen (d15N), oxygen (d18O), and bulk boron (d11B) isotope ratios to identify sources of nitrate-contaminated waters: a guideline to identify polluters

Jan Bronders, Kristof Tirez, Nele Desmet, David Widory, Emmanuelle Petelet-Giraud, Agnès Bregnot and Pascal Boeckx UGent (2012) ENVIRONMENTAL FORENSICS. 13(1). p.32-38
abstract
The use of various isotopes (d(15)N, d(18)O & d(11)B) to identify the sources of nitrate (NO3-) present in natural waters is described. Then a new guideline of how to apply the multi-isotope approach is presented. This guideline is written for policy makers and scientists who are involved in the different steps and processes related to nitrate contaminated waters including monitoring and data interpretation. NO3- is a common pollutant in water (both surface and groundwater). In several water bodies over Europe, point measurements identify that the level of this pollutant is higher than the reference value of 50 mgL(-1), defined by the European Union (EU) Water Framework Directive 2000/60/EC (European Parliament, 2000). This directive also states that all waters have to reach a "good status" (i.e., good quality) by 2015. This statement implies that EU member states have to take actions to achieve this goal. One of the major obstacles with NO3- contamination in water is the identification of the corresponding source(s) of pollution, a prerequisite for properly designing appropriate actions and remediation. Recent studies have proven the added value of analyzing compound specific isotopic signature (CSIA) of nitrate (both nitrogen (d(15)N), oxygen (d(18)O) and bulk boron (d(11)B) isotopic composition) to define the origin/source of NO3- in waters. This definition is possible because different sources of nitrate have distinct isotopic signatures. The recent EU-LIFE ISONITRATE project demonstrated the benefit of the multi-isotope approach, while the presented guideline to implement this method is one of the outcomes of this project. More details on the scientific results of ISONITRATE are available at http://isonitrate.brgm.fr/.
Please use this url to cite or link to this publication:
author
organization
alternative title
Use of compound-specific nitrogen (d(15)N), oxygen (d(18)O), and bulk boron (d(11)B) isotope ratios to identify sources of nitrate-contaminated waters : a guideline to identify polluters
year
type
journalArticle (original)
publication status
published
subject
keyword
isotopes, nitrate, nitrogen, oxygen, boron, nitrate sources, STABLE-ISOTOPES, GROUNDWATER, RIVER, UNCERTAINTY
journal title
ENVIRONMENTAL FORENSICS
Environ. Forensics
volume
13
issue
1
pages
32 - 38
Web of Science type
Article
Web of Science id
000305175000004
JCR category
ENVIRONMENTAL SCIENCES
JCR impact factor
0.652 (2012)
JCR rank
180/209 (2012)
JCR quartile
4 (2012)
ISSN
1527-5922
DOI
10.1080/15275922.2011.643338
language
English
UGent publication?
yes
classification
A1
copyright statement
I have transferred the copyright for this publication to the publisher
id
3191292
handle
http://hdl.handle.net/1854/LU-3191292
date created
2013-04-11 10:16:03
date last changed
2016-12-19 15:38:06
@article{3191292,
  abstract     = {The use of various isotopes (d(15)N, d(18)O \& d(11)B) to identify the sources of nitrate (NO3-) present in natural waters is described. Then a new guideline of how to apply the multi-isotope approach is presented. This guideline is written for policy makers and scientists who are involved in the different steps and processes related to nitrate contaminated waters including monitoring and data interpretation. NO3- is a common pollutant in water (both surface and groundwater). In several water bodies over Europe, point measurements identify that the level of this pollutant is higher than the reference value of 50 mgL(-1), defined by the European Union (EU) Water Framework Directive 2000/60/EC (European Parliament, 2000). This directive also states that all waters have to reach a {\textacutedbl}good status{\textacutedbl} (i.e., good quality) by 2015. This statement implies that EU member states have to take actions to achieve this goal. One of the major obstacles with NO3- contamination in water is the identification of the corresponding source(s) of pollution, a prerequisite for properly designing appropriate actions and remediation. Recent studies have proven the added value of analyzing compound specific isotopic signature (CSIA) of nitrate (both nitrogen (d(15)N), oxygen (d(18)O) and bulk boron (d(11)B) isotopic composition) to define the origin/source of NO3- in waters. This definition is possible because different sources of nitrate have distinct isotopic signatures. The recent EU-LIFE ISONITRATE project demonstrated the benefit of the multi-isotope approach, while the presented guideline to implement this method is one of the outcomes of this project. More details on the scientific results of ISONITRATE are available at http://isonitrate.brgm.fr/.},
  author       = {Bronders, Jan and Tirez, Kristof and Desmet, Nele and Widory, David and Petelet-Giraud, Emmanuelle and Bregnot, Agn{\`e}s and Boeckx, Pascal},
  issn         = {1527-5922},
  journal      = {ENVIRONMENTAL FORENSICS},
  keyword      = {isotopes,nitrate,nitrogen,oxygen,boron,nitrate sources,STABLE-ISOTOPES,GROUNDWATER,RIVER,UNCERTAINTY},
  language     = {eng},
  number       = {1},
  pages        = {32--38},
  title        = {Use of compound-specific nitrogen (d15N), oxygen (d18O), and bulk boron (d11B) isotope ratios to identify sources of nitrate-contaminated waters: a guideline to identify polluters},
  url          = {http://dx.doi.org/10.1080/15275922.2011.643338},
  volume       = {13},
  year         = {2012},
}

Chicago
Bronders, Jan, Kristof Tirez, Nele Desmet, David Widory, Emmanuelle Petelet-Giraud, Agnès Bregnot, and Pascal Boeckx. 2012. “Use of Compound-specific Nitrogen (d15N), Oxygen (d18O), and Bulk Boron (d11B) Isotope Ratios to Identify Sources of Nitrate-contaminated Waters: a Guideline to Identify Polluters.” Environmental Forensics 13 (1): 32–38.
APA
Bronders, J., Tirez, K., Desmet, N., Widory, D., Petelet-Giraud, E., Bregnot, A., & Boeckx, P. (2012). Use of compound-specific nitrogen (d15N), oxygen (d18O), and bulk boron (d11B) isotope ratios to identify sources of nitrate-contaminated waters: a guideline to identify polluters. ENVIRONMENTAL FORENSICS, 13(1), 32–38.
Vancouver
1.
Bronders J, Tirez K, Desmet N, Widory D, Petelet-Giraud E, Bregnot A, et al. Use of compound-specific nitrogen (d15N), oxygen (d18O), and bulk boron (d11B) isotope ratios to identify sources of nitrate-contaminated waters: a guideline to identify polluters. ENVIRONMENTAL FORENSICS. 2012;13(1):32–8.
MLA
Bronders, Jan, Kristof Tirez, Nele Desmet, et al. “Use of Compound-specific Nitrogen (d15N), Oxygen (d18O), and Bulk Boron (d11B) Isotope Ratios to Identify Sources of Nitrate-contaminated Waters: a Guideline to Identify Polluters.” ENVIRONMENTAL FORENSICS 13.1 (2012): 32–38. Print.