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An experimental and kinetic modeling study of pyrolysis and combustion af acetone-butanol-ethanol (abe) mixtures

Kevin Van Geem (UGent) , Alberto Cuoci, Alessio Frassoldati, Steven Pyl (UGent) , Guy Marin (UGent) and Eliseo Ranzi
(2012) COMBUSTION SCIENCE AND TECHNOLOGY. 184(7-8). p.942-955
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Abstract
The excellent fuel characteristics of bio-butanol are responsible for the renewed interest in the acetone-butanol-ethanol (ABE) fermentation process and the combustion and pyrolysis behavior of mixtures of acetone, butanol, and ethanol. Therefore, in this work, a detailed mechanism for the pyrolysis and oxidation of ABE is presented containing similar to 350 species and more than 10,000 reactions. The mechanism is validated against newly acquired and published pyrolysis data for the ABE-mixture and the respective components. Excellent agreement is obtained between measured and simulated product yields as a function of the conversion. Laminar flame speed computations of alcohols and ABE complement the detailed comparisons of the pyrolysis data and allow for further validation of the combustion behavior of bio-butanol and its mixtures.
Keywords
SURROGATE MIXTURES, FLAME PROPAGATION, N-PROPANOL, SHOCK-TUBE, OXIDATION, ISOPROPANOL, REDUCTION, IGNITION, SPEEDS, ABE mixtures, Alcohol fuels, Biobutanol, Detailed kinetics, Pyrolysis and combustion

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Citation

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MLA
Van Geem, Kevin, et al. “An Experimental and Kinetic Modeling Study of Pyrolysis and Combustion Af Acetone-Butanol-Ethanol (Abe) Mixtures.” COMBUSTION SCIENCE AND TECHNOLOGY, vol. 184, no. 7–8, 2012, pp. 942–55, doi:10.1080/00102202.2012.663987.
APA
Van Geem, K., Cuoci, A., Frassoldati, A., Pyl, S., Marin, G., & Ranzi, E. (2012). An experimental and kinetic modeling study of pyrolysis and combustion af acetone-butanol-ethanol (abe) mixtures. COMBUSTION SCIENCE AND TECHNOLOGY, 184(7–8), 942–955. https://doi.org/10.1080/00102202.2012.663987
Chicago author-date
Van Geem, Kevin, Alberto Cuoci, Alessio Frassoldati, Steven Pyl, Guy Marin, and Eliseo Ranzi. 2012. “An Experimental and Kinetic Modeling Study of Pyrolysis and Combustion Af Acetone-Butanol-Ethanol (Abe) Mixtures.” COMBUSTION SCIENCE AND TECHNOLOGY 184 (7–8): 942–55. https://doi.org/10.1080/00102202.2012.663987.
Chicago author-date (all authors)
Van Geem, Kevin, Alberto Cuoci, Alessio Frassoldati, Steven Pyl, Guy Marin, and Eliseo Ranzi. 2012. “An Experimental and Kinetic Modeling Study of Pyrolysis and Combustion Af Acetone-Butanol-Ethanol (Abe) Mixtures.” COMBUSTION SCIENCE AND TECHNOLOGY 184 (7–8): 942–955. doi:10.1080/00102202.2012.663987.
Vancouver
1.
Van Geem K, Cuoci A, Frassoldati A, Pyl S, Marin G, Ranzi E. An experimental and kinetic modeling study of pyrolysis and combustion af acetone-butanol-ethanol (abe) mixtures. COMBUSTION SCIENCE AND TECHNOLOGY. 2012;184(7–8):942–55.
IEEE
[1]
K. Van Geem, A. Cuoci, A. Frassoldati, S. Pyl, G. Marin, and E. Ranzi, “An experimental and kinetic modeling study of pyrolysis and combustion af acetone-butanol-ethanol (abe) mixtures,” COMBUSTION SCIENCE AND TECHNOLOGY, vol. 184, no. 7–8, pp. 942–955, 2012.
@article{2969553,
  abstract     = {{The excellent fuel characteristics of bio-butanol are responsible for the renewed interest in the acetone-butanol-ethanol (ABE) fermentation process and the combustion and pyrolysis behavior of mixtures of acetone, butanol, and ethanol. Therefore, in this work, a detailed mechanism for the pyrolysis and oxidation of ABE is presented containing similar to 350 species and more than 10,000 reactions. The mechanism is validated against newly acquired and published pyrolysis data for the ABE-mixture and the respective components. Excellent agreement is obtained between measured and simulated product yields as a function of the conversion. Laminar flame speed computations of alcohols and ABE complement the detailed comparisons of the pyrolysis data and allow for further validation of the combustion behavior of bio-butanol and its mixtures.}},
  author       = {{Van Geem, Kevin and Cuoci, Alberto and Frassoldati, Alessio and Pyl, Steven and Marin, Guy and Ranzi, Eliseo}},
  issn         = {{0010-2202}},
  journal      = {{COMBUSTION SCIENCE AND TECHNOLOGY}},
  keywords     = {{SURROGATE MIXTURES,FLAME PROPAGATION,N-PROPANOL,SHOCK-TUBE,OXIDATION,ISOPROPANOL,REDUCTION,IGNITION,SPEEDS,ABE mixtures,Alcohol fuels,Biobutanol,Detailed kinetics,Pyrolysis and combustion}},
  language     = {{eng}},
  number       = {{7-8}},
  pages        = {{942--955}},
  title        = {{An experimental and kinetic modeling study of pyrolysis and combustion af acetone-butanol-ethanol (abe) mixtures}},
  url          = {{http://dx.doi.org/10.1080/00102202.2012.663987}},
  volume       = {{184}},
  year         = {{2012}},
}
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