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An experimental and kinetic modeling study of pyrolysis and combustion af acetone-butanol-ethanol (abe) mixtures

Kevin Van Geem UGent, Alberto Cuoci, Alessio Frassoldati, Steven Pyl UGent, Guy Marin UGent and Eliseo Ranzi (2012) COMBUSTION SCIENCE AND TECHNOLOGY. 184(7-8). p.942-955
abstract
The excellent fuel characteristics of bio-butanol are responsible for the renewed interest in the acetone-butanol-ethanol (ABE) fermentation process and the combustion and pyrolysis behavior of mixtures of acetone, butanol, and ethanol. Therefore, in this work, a detailed mechanism for the pyrolysis and oxidation of ABE is presented containing similar to 350 species and more than 10,000 reactions. The mechanism is validated against newly acquired and published pyrolysis data for the ABE-mixture and the respective components. Excellent agreement is obtained between measured and simulated product yields as a function of the conversion. Laminar flame speed computations of alcohols and ABE complement the detailed comparisons of the pyrolysis data and allow for further validation of the combustion behavior of bio-butanol and its mixtures.
Please use this url to cite or link to this publication:
author
organization
year
type
journalArticle (original)
publication status
published
subject
keyword
SURROGATE MIXTURES, FLAME PROPAGATION, N-PROPANOL, SHOCK-TUBE, OXIDATION, ISOPROPANOL, REDUCTION, IGNITION, SPEEDS, ABE mixtures, Alcohol fuels, Biobutanol, Detailed kinetics, Pyrolysis and combustion
journal title
COMBUSTION SCIENCE AND TECHNOLOGY
Combust. Sci. Technol.
volume
184
issue
7-8
issue title
Seventh Mediterranean Combustion Symposium
pages
942 - 955
Web of Science type
Article
Web of Science id
000307190700007
JCR category
ENGINEERING, MULTIDISCIPLINARY
JCR impact factor
1.011 (2012)
JCR rank
33/88 (2012)
JCR quartile
2 (2012)
ISSN
0010-2202
DOI
10.1080/00102202.2012.663987
project
Biotechnology for a sustainable economy (Bio-Economy)
language
English
UGent publication?
yes
classification
A1
copyright statement
I have transferred the copyright for this publication to the publisher
id
2969553
handle
http://hdl.handle.net/1854/LU-2969553
date created
2012-08-07 16:11:26
date last changed
2014-05-26 10:04:21
@article{2969553,
  abstract     = {The excellent fuel characteristics of bio-butanol are responsible for the renewed interest in the acetone-butanol-ethanol (ABE) fermentation process and the combustion and pyrolysis behavior of mixtures of acetone, butanol, and ethanol. Therefore, in this work, a detailed mechanism for the pyrolysis and oxidation of ABE is presented containing similar to 350 species and more than 10,000 reactions. The mechanism is validated against newly acquired and published pyrolysis data for the ABE-mixture and the respective components. Excellent agreement is obtained between measured and simulated product yields as a function of the conversion. Laminar flame speed computations of alcohols and ABE complement the detailed comparisons of the pyrolysis data and allow for further validation of the combustion behavior of bio-butanol and its mixtures.},
  author       = {Van Geem, Kevin and Cuoci, Alberto and Frassoldati, Alessio and Pyl, Steven and Marin, Guy and Ranzi, Eliseo},
  issn         = {0010-2202},
  journal      = {COMBUSTION SCIENCE AND TECHNOLOGY},
  keyword      = {SURROGATE MIXTURES,FLAME PROPAGATION,N-PROPANOL,SHOCK-TUBE,OXIDATION,ISOPROPANOL,REDUCTION,IGNITION,SPEEDS,ABE mixtures,Alcohol fuels,Biobutanol,Detailed kinetics,Pyrolysis and combustion},
  language     = {eng},
  number       = {7-8},
  pages        = {942--955},
  title        = {An experimental and kinetic modeling study of pyrolysis and combustion af acetone-butanol-ethanol (abe) mixtures},
  url          = {http://dx.doi.org/10.1080/00102202.2012.663987},
  volume       = {184},
  year         = {2012},
}

Chicago
Van Geem, Kevin, Alberto Cuoci, Alessio Frassoldati, Steven Pyl, Guy Marin, and Eliseo Ranzi. 2012. “An Experimental and Kinetic Modeling Study of Pyrolysis and Combustion Af Acetone-butanol-ethanol (abe) Mixtures.” Combustion Science and Technology 184 (7-8): 942–955.
APA
Van Geem, K., Cuoci, A., Frassoldati, A., Pyl, S., Marin, G., & Ranzi, E. (2012). An experimental and kinetic modeling study of pyrolysis and combustion af acetone-butanol-ethanol (abe) mixtures. COMBUSTION SCIENCE AND TECHNOLOGY, 184(7-8), 942–955.
Vancouver
1.
Van Geem K, Cuoci A, Frassoldati A, Pyl S, Marin G, Ranzi E. An experimental and kinetic modeling study of pyrolysis and combustion af acetone-butanol-ethanol (abe) mixtures. COMBUSTION SCIENCE AND TECHNOLOGY. 2012;184(7-8):942–55.
MLA
Van Geem, Kevin, Alberto Cuoci, Alessio Frassoldati, et al. “An Experimental and Kinetic Modeling Study of Pyrolysis and Combustion Af Acetone-butanol-ethanol (abe) Mixtures.” COMBUSTION SCIENCE AND TECHNOLOGY 184.7-8 (2012): 942–955. Print.