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Plasma polymerisation of siloxanes at atmospheric pressure

Nathalie De Geyter UGent, Rino Morent UGent, Sandra Van Vlierberghe UGent, Peter Dubruel UGent, Christophe Leys UGent and Etienne Schacht UGent (2011) SURFACE ENGINEERING. 27(8). p.627-633
abstract
This work deals with the plasma polymerisation of two siloxane precursors, [hexamethyldisiloxane (HMDSO) and tetramethyldisiloxane (TMDSO)] with an atmospheric pressure pseudoglow dielectric barrier discharge operated in argon and an argon-air mixture. The influence of gas composition and precursor type on the physical and chemical properties of the deposited films is examined in detail using contact angle measurements, Fourier transform infrared spectroscopy (FTIR) and atomic force microscopy (AFM). Results clearly show that precursor type as well as gas composition has an profound impact on film growth rate and chemical composition of the deposited films. Plasma polymerisation of both siloxane precursors in argon leads to the formation of hydrophobic polymers consisting of a Si-O-Si backbone, while for deposition in an argon-air mixture, hydrophilic inorganic silica-like coatings are obtained.
Please use this url to cite or link to this publication:
author
organization
year
type
journalArticle (original)
publication status
published
subject
keyword
Tetramethyldisiloxane, Dielectric barrier discharge, POLYETHYLENE TEREPHTHALATE, Atmospheric pressure, SURFACE-TREATMENT, THIN-FILMS, GLOW-DISCHARGE, DIELECTRIC BARRIER DISCHARGE, SIOX FILMS, DEPOSITION, HELIUM, COATINGS, TETRAETHOXYSILANE, Hexamethyldisiloxane, Plasma polymerisation
journal title
SURFACE ENGINEERING
Surf. Eng.
volume
27
issue
8
pages
627 - 633
Web of Science type
Article
Web of Science id
000296566800012
JCR category
MATERIALS SCIENCE, COATINGS & FILMS
JCR impact factor
0.937 (2011)
JCR rank
11/18 (2011)
JCR quartile
3 (2011)
ISSN
0267-0844
DOI
10.1179/174329409X433858
language
English
UGent publication?
yes
classification
A1
copyright statement
I have transferred the copyright for this publication to the publisher
id
2957043
handle
http://hdl.handle.net/1854/LU-2957043
date created
2012-07-06 11:30:48
date last changed
2012-07-30 10:02:31
@article{2957043,
  abstract     = {This work deals with the plasma polymerisation of two siloxane precursors, [hexamethyldisiloxane (HMDSO) and tetramethyldisiloxane (TMDSO)] with an atmospheric pressure pseudoglow dielectric barrier discharge operated in argon and an argon-air mixture. The influence of gas composition and precursor type on the physical and chemical properties of the deposited films is examined in detail using contact angle measurements, Fourier transform infrared spectroscopy (FTIR) and atomic force microscopy (AFM). Results clearly show that precursor type as well as gas composition has an profound impact on film growth rate and chemical composition of the deposited films. Plasma polymerisation of both siloxane precursors in argon leads to the formation of hydrophobic polymers consisting of a Si-O-Si backbone, while for deposition in an argon-air mixture, hydrophilic inorganic silica-like coatings are obtained.},
  author       = {De Geyter, Nathalie and Morent, Rino and Van Vlierberghe, Sandra and Dubruel, Peter and Leys, Christophe and Schacht, Etienne},
  issn         = {0267-0844},
  journal      = {SURFACE ENGINEERING},
  keyword      = {Tetramethyldisiloxane,Dielectric barrier discharge,POLYETHYLENE TEREPHTHALATE,Atmospheric pressure,SURFACE-TREATMENT,THIN-FILMS,GLOW-DISCHARGE,DIELECTRIC BARRIER DISCHARGE,SIOX FILMS,DEPOSITION,HELIUM,COATINGS,TETRAETHOXYSILANE,Hexamethyldisiloxane,Plasma polymerisation},
  language     = {eng},
  number       = {8},
  pages        = {627--633},
  title        = {Plasma polymerisation of siloxanes at atmospheric pressure},
  url          = {http://dx.doi.org/10.1179/174329409X433858},
  volume       = {27},
  year         = {2011},
}

Chicago
De Geyter, Nathalie, Rino Morent, Sandra Van Vlierberghe, Peter Dubruel, Christophe Leys, and Etienne Schacht. 2011. “Plasma Polymerisation of Siloxanes at Atmospheric Pressure.” Surface Engineering 27 (8): 627–633.
APA
De Geyter, N., Morent, R., Van Vlierberghe, S., Dubruel, P., Leys, C., & Schacht, E. (2011). Plasma polymerisation of siloxanes at atmospheric pressure. SURFACE ENGINEERING, 27(8), 627–633.
Vancouver
1.
De Geyter N, Morent R, Van Vlierberghe S, Dubruel P, Leys C, Schacht E. Plasma polymerisation of siloxanes at atmospheric pressure. SURFACE ENGINEERING. 2011;27(8):627–33.
MLA
De Geyter, Nathalie, Rino Morent, Sandra Van Vlierberghe, et al. “Plasma Polymerisation of Siloxanes at Atmospheric Pressure.” SURFACE ENGINEERING 27.8 (2011): 627–633. Print.