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Qualitative by-product identification of plasma-assisted TCE abatement by mass spectrometry and Fourier-transform infrared spectroscopy

Arne Vandenbroucke, Minh Tuan Nguyen Dinh , Jean-Marc Giraudon, Rino Morent UGent, Nathalie De Geyter UGent, Jean-Francois Lamonier and Christophe Leys UGent (2011) PLASMA CHEMISTRY AND PLASMA PROCESSING. 31(5). p.707-718
abstract
In this study, the formation of by-products resulting from the decomposition of trichloroethylene with a negative DC glow discharge has been investigated. By combining the qualitative data from mass spectrometry and Fourier-transform infrared spectroscopy, the formation of phosgene, dichloroacetylchloride and trichloroacetaldehyde have been confirmed as incomplete oxidation products. Hydrogen chloride, chlorine, carbon monoxide and carbon dioxide were also detected. Also, formation of ozone was found in the outlet stream. Based on this information, it is possible to chose an appropriate catalyst to combine with non thermal plasma. In this way emission of harmful, incomplete oxidation products can be further reduced at a lower energy cost.
Please use this url to cite or link to this publication:
author
organization
year
type
journalArticle (original)
publication status
published
subject
keyword
AIR-POLLUTION CONTROL, WASTE-GAS TREATMENT, VOLATILE ORGANIC-COMPOUNDS, NONTHERMAL PLASMA, ELECTRICAL-DISCHARGE, ATMOSPHERIC-PRESSURE, CATALYTIC COMBUSTION, GLOW-DISCHARGE, DECOMPOSITION, REMOVAL, Non-thermal plasma, VOC, Negative DC glow discharge, By-products, FT-IR, MS
journal title
PLASMA CHEMISTRY AND PLASMA PROCESSING
Plasma Chem. Plasma Process.
volume
31
issue
5
pages
707 - 718
Web of Science type
Article
Web of Science id
000300100900006
ISSN
1572-8986
DOI
10.1007/s11090-011-9310-7
language
English
UGent publication?
yes
classification
A1
copyright statement
I have transferred the copyright for this publication to the publisher
id
1910309
handle
http://hdl.handle.net/1854/LU-1910309
date created
2011-09-28 11:04:47
date last changed
2016-12-19 15:46:25
@article{1910309,
  abstract     = {In this study, the formation of by-products resulting from the decomposition of trichloroethylene with a negative DC glow discharge has been investigated. By combining the qualitative data from mass spectrometry and Fourier-transform infrared spectroscopy, the formation of phosgene, dichloroacetylchloride and trichloroacetaldehyde have been confirmed as incomplete oxidation products. Hydrogen chloride, chlorine, carbon monoxide and carbon dioxide were also detected. Also, formation of ozone was found in the outlet stream. Based on this information, it is possible to chose an appropriate catalyst to combine with non thermal plasma. In this way emission of harmful, incomplete oxidation products can be further reduced at a lower energy cost.},
  author       = {Vandenbroucke, Arne and Nguyen Dinh , Minh Tuan  and Giraudon, Jean-Marc  and Morent, Rino and De Geyter, Nathalie and Lamonier, Jean-Francois  and Leys, Christophe},
  issn         = {1572-8986},
  journal      = {PLASMA CHEMISTRY AND PLASMA PROCESSING},
  keyword      = {AIR-POLLUTION CONTROL,WASTE-GAS TREATMENT,VOLATILE ORGANIC-COMPOUNDS,NONTHERMAL PLASMA,ELECTRICAL-DISCHARGE,ATMOSPHERIC-PRESSURE,CATALYTIC COMBUSTION,GLOW-DISCHARGE,DECOMPOSITION,REMOVAL,Non-thermal plasma,VOC,Negative DC glow discharge,By-products,FT-IR,MS},
  language     = {eng},
  number       = {5},
  pages        = {707--718},
  title        = {Qualitative by-product identification of plasma-assisted TCE abatement by mass spectrometry and Fourier-transform infrared spectroscopy},
  url          = {http://dx.doi.org/10.1007/s11090-011-9310-7},
  volume       = {31},
  year         = {2011},
}

Chicago
Vandenbroucke, Arne, Minh Tuan Nguyen Dinh , Jean-Marc Giraudon, Rino Morent, Nathalie De Geyter, Jean-Francois Lamonier, and Christophe Leys. 2011. “Qualitative By-product Identification of Plasma-assisted TCE Abatement by Mass Spectrometry and Fourier-transform Infrared Spectroscopy.” Plasma Chemistry and Plasma Processing 31 (5): 707–718.
APA
Vandenbroucke, Arne, Nguyen Dinh , M. T., Giraudon, J.-M., Morent, R., De Geyter, N., Lamonier, J.-F., & Leys, C. (2011). Qualitative by-product identification of plasma-assisted TCE abatement by mass spectrometry and Fourier-transform infrared spectroscopy. PLASMA CHEMISTRY AND PLASMA PROCESSING, 31(5), 707–718.
Vancouver
1.
Vandenbroucke A, Nguyen Dinh MT, Giraudon J-M, Morent R, De Geyter N, Lamonier J-F, et al. Qualitative by-product identification of plasma-assisted TCE abatement by mass spectrometry and Fourier-transform infrared spectroscopy. PLASMA CHEMISTRY AND PLASMA PROCESSING. 2011;31(5):707–18.
MLA
Vandenbroucke, Arne, Minh Tuan Nguyen Dinh , Jean-Marc Giraudon, et al. “Qualitative By-product Identification of Plasma-assisted TCE Abatement by Mass Spectrometry and Fourier-transform Infrared Spectroscopy.” PLASMA CHEMISTRY AND PLASMA PROCESSING 31.5 (2011): 707–718. Print.