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Single-event microkinetics of hydrocarbon cracking on zeotype catalysts: effect of acidity and shape selectivity

Rhona Van Borm UGent (2011)
abstract
This work fits in the research on the design and optimization of the catalytic cracking of hydrocarbons. Because increasingly heavier petroleum fractions are fed industrially, it is important to rationally design new catalysts with larger pores than the current zeolites. In this respect, it is essential to develop fundamental kinetic models, that can account for the effect of catalyst properties such as acidity and shape selectivity on the catalytic behavior. In this work, the effect of these catalyst properties on the activity and selectivity is studied experimentally on a series of commercial zeolites and on two newly developed zeotype materials with bimodal pore network. Based on these results, accurate and flexible kinetic models are developed that explicitly describe these effects.
Please use this url to cite or link to this publication:
author
promoter
UGent and UGent
organization
alternative title
Single-event microkinetiek van het kraken van koolwaterstoffen over zeotype katalysatoren : effect van zuursterkte en vormselectiviteit
year
type
dissertation (monograph)
subject
keyword
shape selectivity, acidity, hydrocarbons, catalytic cracking, FAU, MFI, kinetics, BIPOMs
pages
XXVIII, 210 pages
publisher
Ghent University. Faculty of Engineering and Architecture
place of publication
Ghent, Belgium
defense location
Gent : Faculteit Ingenieurswetenschappen en Architectuur (Jozef Plateauzaal)
defense date
2011-02-02 16:00
ISBN
9789085784043
language
English
UGent publication?
yes
classification
D1
additional info
dissertation in part contains copyrighted material
copyright statement
I have transferred the copyright for this publication to the publisher
id
1209612
handle
http://hdl.handle.net/1854/LU-1209612
date created
2011-04-17 11:33:38
date last changed
2011-04-18 09:01:05
@phdthesis{1209612,
  abstract     = {This work fits in the research on the design and optimization of the catalytic cracking of hydrocarbons. Because increasingly heavier petroleum fractions are fed industrially, it is important to rationally design new catalysts with larger pores than the current zeolites. In this respect, it is essential to develop fundamental kinetic models, that can account for the effect of catalyst properties such as acidity and  shape selectivity on the catalytic behavior.
In this work, the effect of these catalyst properties on the activity and selectivity is studied experimentally on a series of commercial zeolites and on two newly developed zeotype materials with bimodal pore network. Based on these results, accurate and flexible kinetic models are developed that explicitly describe these effects.},
  author       = {Van Borm, Rhona},
  isbn         = {9789085784043},
  keyword      = {shape selectivity,acidity,hydrocarbons,catalytic cracking,FAU,MFI,kinetics,BIPOMs},
  language     = {eng},
  pages        = {XXVIII, 210},
  publisher    = {Ghent University. Faculty of Engineering and Architecture},
  school       = {Ghent University},
  title        = {Single-event microkinetics of hydrocarbon cracking on zeotype catalysts: effect of acidity and shape selectivity},
  year         = {2011},
}

Chicago
Van Borm, Rhona. 2011. “Single-event Microkinetics of Hydrocarbon Cracking on Zeotype Catalysts: Effect of Acidity and Shape Selectivity”. Ghent, Belgium: Ghent University. Faculty of Engineering and Architecture.
APA
Van Borm, R. (2011). Single-event microkinetics of hydrocarbon cracking on zeotype catalysts: effect of acidity and shape selectivity. Ghent University. Faculty of Engineering and Architecture, Ghent, Belgium.
Vancouver
1.
Van Borm R. Single-event microkinetics of hydrocarbon cracking on zeotype catalysts: effect of acidity and shape selectivity. [Ghent, Belgium]: Ghent University. Faculty of Engineering and Architecture; 2011.
MLA
Van Borm, Rhona. “Single-event Microkinetics of Hydrocarbon Cracking on Zeotype Catalysts: Effect of Acidity and Shape Selectivity.” 2011 : n. pag. Print.