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Process intensification of solid‐sorbent DAC via a rotating vortex reactor

Afroditi Kourou (UGent) , Siyuan Chen (UGent) , Bing Wang (UGent) , Geraldine Heynderickx (UGent) , Kevin Van Geem (UGent) and Yi Ouyang (UGent)
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Abstract
This work investigates the performance of the rotating vortex reactor (RVR) as a promising intensified contactor for direct air capture (DAC). Both adsorption and desorption are tested across ranges of superficial gas velocities and rotation speeds, thereby tuning the bed regime—packed or fluidized—under a centrifugal force field (known as a high‐gravity condition) and a vortex flow to enhance mass and heat transfer. A cyclic cut‐off analysis further quantifies the contributions of the main energy consumers and clarifies the trade‐offs between productivity and energy demand. The adsorber achieves high volumetric CO2, while hot‐air regeneration enables rapid desorption in <10 min. This proof‐of‐concept study shows RVR's potential for process intensification while identifying areas for further improvement in the unit's design and operation to reduce energy demand for DAC.
Keywords
contactor design, direct air capture, high-gravity vortex technology, process intensification, rotating vortex reactor, DIRECT AIR CAPTURE, FLUIDIZED-BED, CO2 CAPTURE, ADSORPTION

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MLA
Kourou, Afroditi, et al. “Process Intensification of Solid‐sorbent DAC via a Rotating Vortex Reactor.” AICHE JOURNAL, 2026, doi:10.1002/aic.70421.
APA
Kourou, A., Chen, S., Wang, B., Heynderickx, G., Van Geem, K., & Ouyang, Y. (2026). Process intensification of solid‐sorbent DAC via a rotating vortex reactor. AICHE JOURNAL. https://doi.org/10.1002/aic.70421
Chicago author-date
Kourou, Afroditi, Siyuan Chen, Bing Wang, Geraldine Heynderickx, Kevin Van Geem, and Yi Ouyang. 2026. “Process Intensification of Solid‐sorbent DAC via a Rotating Vortex Reactor.” AICHE JOURNAL. https://doi.org/10.1002/aic.70421.
Chicago author-date (all authors)
Kourou, Afroditi, Siyuan Chen, Bing Wang, Geraldine Heynderickx, Kevin Van Geem, and Yi Ouyang. 2026. “Process Intensification of Solid‐sorbent DAC via a Rotating Vortex Reactor.” AICHE JOURNAL. doi:10.1002/aic.70421.
Vancouver
1.
Kourou A, Chen S, Wang B, Heynderickx G, Van Geem K, Ouyang Y. Process intensification of solid‐sorbent DAC via a rotating vortex reactor. AICHE JOURNAL. 2026;
IEEE
[1]
A. Kourou, S. Chen, B. Wang, G. Heynderickx, K. Van Geem, and Y. Ouyang, “Process intensification of solid‐sorbent DAC via a rotating vortex reactor,” AICHE JOURNAL, 2026.
@article{01KT3WJDZ7EN1ECD7BP99SNBNF,
  abstract     = {{This work investigates the performance of the rotating vortex reactor (RVR) as a promising intensified contactor for direct air capture (DAC). Both adsorption and desorption are tested across ranges of superficial gas velocities and rotation speeds, thereby tuning the bed regime—packed or fluidized—under a centrifugal force field (known as a high‐gravity condition) and a vortex flow to enhance mass and heat transfer. A cyclic cut‐off analysis further quantifies the contributions of the main energy consumers and clarifies the trade‐offs between productivity and energy demand. The adsorber achieves high volumetric CO2, while hot‐air regeneration enables rapid desorption in <10 min. This proof‐of‐concept study shows RVR's potential for process intensification while identifying areas for further improvement in the unit's design and operation to reduce energy demand for DAC.}},
  articleno    = {{e70421}},
  author       = {{Kourou, Afroditi and Chen, Siyuan and Wang, Bing and Heynderickx, Geraldine and Van Geem, Kevin and Ouyang, Yi}},
  issn         = {{0001-1541}},
  journal      = {{AICHE JOURNAL}},
  keywords     = {{contactor design,direct air capture,high-gravity vortex technology,process intensification,rotating vortex reactor,DIRECT AIR CAPTURE,FLUIDIZED-BED,CO2 CAPTURE,ADSORPTION}},
  language     = {{eng}},
  pages        = {{14}},
  title        = {{Process intensification of solid‐sorbent DAC via a rotating vortex reactor}},
  url          = {{http://doi.org/10.1002/aic.70421}},
  year         = {{2026}},
}

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