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Rapid one-step synthesis of robust double perovskite La2MgGeO6-based materials for light conversion

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Abstract
Persistent luminescence (PersL) materials attract extensive interest in the scientific community nowadays due to their great potential in various fields, such as night-vision signage, high-level anticounterfeiting, in vivo bioimaging, and X-ray extension imaging. However, the majority of PersL materials are synthesized by time- and energy-consuming processes such as high-temperature solid-state reactions or hydrothermal synthesis. In this work, a rapid one-step microwave-assisted solid state (MASS) synthesis of La2MgGeO6-based robust double perovskite PersL material is successfully achieved, without any secondary thermal treatment, which limits the total synthesis time to 30 min. Furthermore, this MASS approach is also employed to integrate multimodal luminescence into one single La2MgGeO6 matrix with triple dopants (Mn4+, Yb3+, and Er3+) for light conversion. Impressively, multimodal and multicolor luminescence is obtained with different responsiveness of external stimulations. Notably, the energy transfer among different trapping levels is observed upon photo-stimulation. This work provides a good example of the feasibility of MASS method to prepare luminescent materials with abundant optical features in an efficient, sustainable, environmentally friendly, and easily manageable way.
Keywords
microwave assisted synthesis, La2MgGeO6, persistent luminescence, double perovskite, PERSISTENT LUMINESCENCE, TEMPERATURE, MECHANISM, STORAGE, ROUTE

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MLA
Zhang, Jiaping, et al. “Rapid One-Step Synthesis of Robust Double Perovskite La2MgGeO6-Based Materials for Light Conversion.” ADVANCED SUSTAINABLE SYSTEMS, vol. 8, no. 10, 2024, doi:10.1002/adsu.202400285.
APA
Zhang, J., Li, Y., Lin, H., Poelman, D., & Du, J. (2024). Rapid one-step synthesis of robust double perovskite La2MgGeO6-based materials for light conversion. ADVANCED SUSTAINABLE SYSTEMS, 8(10). https://doi.org/10.1002/adsu.202400285
Chicago author-date
Zhang, Jiaping, Yukun Li, Hengwei Lin, Dirk Poelman, and Jiaren Du. 2024. “Rapid One-Step Synthesis of Robust Double Perovskite La2MgGeO6-Based Materials for Light Conversion.” ADVANCED SUSTAINABLE SYSTEMS 8 (10). https://doi.org/10.1002/adsu.202400285.
Chicago author-date (all authors)
Zhang, Jiaping, Yukun Li, Hengwei Lin, Dirk Poelman, and Jiaren Du. 2024. “Rapid One-Step Synthesis of Robust Double Perovskite La2MgGeO6-Based Materials for Light Conversion.” ADVANCED SUSTAINABLE SYSTEMS 8 (10). doi:10.1002/adsu.202400285.
Vancouver
1.
Zhang J, Li Y, Lin H, Poelman D, Du J. Rapid one-step synthesis of robust double perovskite La2MgGeO6-based materials for light conversion. ADVANCED SUSTAINABLE SYSTEMS. 2024;8(10).
IEEE
[1]
J. Zhang, Y. Li, H. Lin, D. Poelman, and J. Du, “Rapid one-step synthesis of robust double perovskite La2MgGeO6-based materials for light conversion,” ADVANCED SUSTAINABLE SYSTEMS, vol. 8, no. 10, 2024.
@article{01J0JZN721RTRAN86N70NPSPDC,
  abstract     = {{Persistent luminescence (PersL) materials attract extensive interest in the scientific community nowadays due to their great potential in various fields, such as night-vision signage, high-level anticounterfeiting, in vivo bioimaging, and X-ray extension imaging. However, the majority of PersL materials are synthesized by time- and energy-consuming processes such as high-temperature solid-state reactions or hydrothermal synthesis. In this work, a rapid one-step microwave-assisted solid state (MASS) synthesis of La2MgGeO6-based robust double perovskite PersL material is successfully achieved, without any secondary thermal treatment, which limits the total synthesis time to 30 min. Furthermore, this MASS approach is also employed to integrate multimodal luminescence into one single La2MgGeO6 matrix with triple dopants (Mn4+, Yb3+, and Er3+) for light conversion. Impressively, multimodal and multicolor luminescence is obtained with different responsiveness of external stimulations. Notably, the energy transfer among different trapping levels is observed upon photo-stimulation. This work provides a good example of the feasibility of MASS method to prepare luminescent materials with abundant optical features in an efficient, sustainable, environmentally friendly, and easily manageable way.}},
  articleno    = {{2400285}},
  author       = {{Zhang, Jiaping and Li, Yukun and  Lin, Hengwei and Poelman, Dirk and Du, Jiaren}},
  issn         = {{2366-7486}},
  journal      = {{ADVANCED SUSTAINABLE SYSTEMS}},
  keywords     = {{microwave assisted synthesis,La2MgGeO6,persistent luminescence,double perovskite,PERSISTENT LUMINESCENCE,TEMPERATURE,MECHANISM,STORAGE,ROUTE}},
  language     = {{eng}},
  number       = {{10}},
  pages        = {{9}},
  title        = {{Rapid one-step synthesis of robust double perovskite La2MgGeO6-based materials for light conversion}},
  url          = {{http://doi.org/10.1002/adsu.202400285}},
  volume       = {{8}},
  year         = {{2024}},
}

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