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Metal-organic frameworks and covalent organic frameworks as photocatalysts for H2O2 production from oxygen and water

Jiamin Sun, Jeet Chakraborty (UGent) , Maojun Deng (UGent) , Andreas Laemont (UGent) , Xiao Feng, Ying-Ya Liu (UGent) and Pascal Van Der Voort (UGent)
(2023) JOURNAL OF MATERIALS CHEMISTRY A. 11(40). p.21516-21540
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Abstract
Hydrogen peroxide (H2O2) plays a vital role in various industries, from healthcare and pharmaceuticals to water treatment and electronics. Its importance lies in its versatility as a powerful and green oxidizing agent and disinfectant. However, with an anticipated increase in demand for H2O2, greener production methods are required. Photocatalytic H2O2 generation (from O2 and/or H2O) using Metal-Organic Frameworks (MOFs) and Covalent Organic Frameworks (COFs) has emerged as a sustainable alternative to traditional methods. This review provides a comprehensive overview of the intrinsic characteristics of MOFs and COFs, focusing on strategies to enhance light harvesting, charge separation, charge mobility, and the associated oxidation and reduction reactions. By addressing current limitations, this review elucidates the fundamental physicochemical properties of these materials, explores H2O2 production mechanisms, and outlines future directions for improved photocatalytic performance.
Keywords
HYDROGEN-PEROXIDE PRODUCTION, TRIAZINE FRAMEWORKS, PHOTOSYNTHESIS, CRYSTALLINE, CENTERS, LIGAND

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MLA
Sun, Jiamin, et al. “Metal-Organic Frameworks and Covalent Organic Frameworks as Photocatalysts for H2O2 Production from Oxygen and Water.” JOURNAL OF MATERIALS CHEMISTRY A, vol. 11, no. 40, 2023, pp. 21516–40, doi:10.1039/d3ta04581a.
APA
Sun, J., Chakraborty, J., Deng, M., Laemont, A., Feng, X., Liu, Y.-Y., & Van Der Voort, P. (2023). Metal-organic frameworks and covalent organic frameworks as photocatalysts for H2O2 production from oxygen and water. JOURNAL OF MATERIALS CHEMISTRY A, 11(40), 21516–21540. https://doi.org/10.1039/d3ta04581a
Chicago author-date
Sun, Jiamin, Jeet Chakraborty, Maojun Deng, Andreas Laemont, Xiao Feng, Ying-Ya Liu, and Pascal Van Der Voort. 2023. “Metal-Organic Frameworks and Covalent Organic Frameworks as Photocatalysts for H2O2 Production from Oxygen and Water.” JOURNAL OF MATERIALS CHEMISTRY A 11 (40): 21516–40. https://doi.org/10.1039/d3ta04581a.
Chicago author-date (all authors)
Sun, Jiamin, Jeet Chakraborty, Maojun Deng, Andreas Laemont, Xiao Feng, Ying-Ya Liu, and Pascal Van Der Voort. 2023. “Metal-Organic Frameworks and Covalent Organic Frameworks as Photocatalysts for H2O2 Production from Oxygen and Water.” JOURNAL OF MATERIALS CHEMISTRY A 11 (40): 21516–21540. doi:10.1039/d3ta04581a.
Vancouver
1.
Sun J, Chakraborty J, Deng M, Laemont A, Feng X, Liu Y-Y, et al. Metal-organic frameworks and covalent organic frameworks as photocatalysts for H2O2 production from oxygen and water. JOURNAL OF MATERIALS CHEMISTRY A. 2023;11(40):21516–40.
IEEE
[1]
J. Sun et al., “Metal-organic frameworks and covalent organic frameworks as photocatalysts for H2O2 production from oxygen and water,” JOURNAL OF MATERIALS CHEMISTRY A, vol. 11, no. 40, pp. 21516–21540, 2023.
@article{01HFMB421FB39NDFJ7QY33KCBH,
  abstract     = {{Hydrogen peroxide (H2O2) plays a vital role in various industries, from

 healthcare and pharmaceuticals to water treatment and electronics. Its

 importance lies in its versatility as a powerful and green oxidizing

 agent and disinfectant. However, with an anticipated increase in demand

 for H2O2, greener production methods are required. Photocatalytic H2O2

 generation (from O2 and/or H2O) using Metal-Organic Frameworks (MOFs)

 and Covalent Organic Frameworks (COFs) has emerged as a sustainable

 alternative to traditional methods. This review provides a comprehensive

 overview of the intrinsic characteristics of MOFs and COFs, focusing on

 strategies to enhance light harvesting, charge separation, charge

 mobility, and the associated oxidation and reduction reactions. By

 addressing current limitations, this review elucidates the fundamental

 physicochemical properties of these materials, explores H2O2 production

 mechanisms, and outlines future directions for improved photocatalytic

 performance.}},
  author       = {{Sun, Jiamin and Chakraborty, Jeet and Deng, Maojun and Laemont, Andreas and Feng, Xiao and Liu, Ying-Ya and Van Der Voort, Pascal}},
  issn         = {{2050-7488}},
  journal      = {{JOURNAL OF MATERIALS CHEMISTRY A}},
  keywords     = {{HYDROGEN-PEROXIDE PRODUCTION,TRIAZINE FRAMEWORKS,PHOTOSYNTHESIS,CRYSTALLINE,CENTERS,LIGAND}},
  language     = {{eng}},
  number       = {{40}},
  pages        = {{21516--21540}},
  title        = {{Metal-organic frameworks and covalent organic frameworks as photocatalysts for H2O2 production from oxygen and water}},
  url          = {{http://doi.org/10.1039/d3ta04581a}},
  volume       = {{11}},
  year         = {{2023}},
}
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