Efficient and sustainable room-temperature CO2 conversion by plasmonic two-dimensional metal-oxide hybrid nano-interfaces
- Author
- Mohammad Karbalaei Akbari, Nasrin Lopa and Serge Zhuiykov (UGent)
- Organization
- Abstract
- The state-of-the-art nanotechnologies ensure the establishment of sustainable green systems for CO2 conversion. Recently, plasmonic two-dimensional (2D) nanostructures are found as effective platforms for efficient visible light-assisted photocatalysis. The plasmonic nanodomains grown on the surface of advanced 2D semiconductor materials represent a new class of hybrid nanostructures. These 2D hybrid nanostructures activate supplementary mechanisms at material heterointerfaces enabling a wide range of solar-activated physic-chemical reactions. Here, the controlled growth of plasmonic crystalline silver (Ag) nanodomains on the 2D surface oxide films of liquid Ga-based nanoparticles enabled the efficient CO2 conversion through combined photocatalysis and acoustic-activated technique. Driven by acoustic energy, the multiple contribution of Ga2O3-Ag semiconductor/plasmonic hybrid 2D heterointerfaces enabled the visible-light assisted hot-electron generation at 2D plasmonic hybridinterfaces and therefore rose the CO2 conversion efficiency to values higher than 94.6%. The inherent plasmonic characteristics of developed 2D nanojunction assembly accompanied by the commercial availability of acoustic activated technologies depict promising future for efficient and sustainable CO2 conversion in industrial levels.
- Keywords
- CO2 Conversion, Two-Dimensional Materials, Plasmonic Photocatalysis, Nanotechnology and Environment
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Please use this url to cite or link to this publication: http://hdl.handle.net/1854/LU-01H8JQZ2PFP803G7P2NGPX327C
- MLA
- Karbalaei Akbari, Mohammad, et al. “Efficient and Sustainable Room-Temperature CO2 Conversion by Plasmonic Two-Dimensional Metal-Oxide Hybrid Nano-Interfaces.” Proceedings of the 7th International Conference of Recent Trends in Environmental Science and Engineering (RTESE’23), 2023, doi:10.11159/rtese23.119.
- APA
- Karbalaei Akbari, M., Lopa, N., & Zhuiykov, S. (2023). Efficient and sustainable room-temperature CO2 conversion by plasmonic two-dimensional metal-oxide hybrid nano-interfaces. Proceedings of the 7th International Conference of Recent Trends in Environmental Science and Engineering (RTESE’23). Presented at the 7th International Conference of Recent Trends in Environmental Science and Engineering, Toronto, Canada. https://doi.org/10.11159/rtese23.119
- Chicago author-date
- Karbalaei Akbari, Mohammad, Nasrin Lopa, and Serge Zhuiykov. 2023. “Efficient and Sustainable Room-Temperature CO2 Conversion by Plasmonic Two-Dimensional Metal-Oxide Hybrid Nano-Interfaces.” In Proceedings of the 7th International Conference of Recent Trends in Environmental Science and Engineering (RTESE’23). https://doi.org/10.11159/rtese23.119.
- Chicago author-date (all authors)
- Karbalaei Akbari, Mohammad, Nasrin Lopa, and Serge Zhuiykov. 2023. “Efficient and Sustainable Room-Temperature CO2 Conversion by Plasmonic Two-Dimensional Metal-Oxide Hybrid Nano-Interfaces.” In Proceedings of the 7th International Conference of Recent Trends in Environmental Science and Engineering (RTESE’23). doi:10.11159/rtese23.119.
- Vancouver
- 1.Karbalaei Akbari M, Lopa N, Zhuiykov S. Efficient and sustainable room-temperature CO2 conversion by plasmonic two-dimensional metal-oxide hybrid nano-interfaces. In: Proceedings of the 7th International Conference of Recent Trends in Environmental Science and Engineering (RTESE’23). 2023.
- IEEE
- [1]M. Karbalaei Akbari, N. Lopa, and S. Zhuiykov, “Efficient and sustainable room-temperature CO2 conversion by plasmonic two-dimensional metal-oxide hybrid nano-interfaces,” in Proceedings of the 7th International Conference of Recent Trends in Environmental Science and Engineering (RTESE’23), Toronto, Canada, 2023.
@inproceedings{01H8JQZ2PFP803G7P2NGPX327C,
abstract = {{The state-of-the-art nanotechnologies ensure the establishment of sustainable green systems for CO2 conversion. Recently, plasmonic two-dimensional (2D) nanostructures are found as effective platforms for efficient visible light-assisted photocatalysis. The plasmonic nanodomains grown on the surface of advanced 2D semiconductor materials represent a new class of hybrid nanostructures. These 2D hybrid nanostructures activate supplementary mechanisms at material heterointerfaces enabling a wide range of solar-activated
physic-chemical reactions. Here, the controlled growth of plasmonic crystalline silver (Ag) nanodomains on the 2D surface oxide films of liquid Ga-based nanoparticles enabled the efficient CO2 conversion through combined photocatalysis and acoustic-activated technique. Driven by acoustic energy, the multiple contribution of Ga2O3-Ag semiconductor/plasmonic hybrid 2D heterointerfaces enabled the visible-light assisted hot-electron generation at 2D plasmonic hybridinterfaces and therefore rose the CO2 conversion efficiency to values higher than 94.6%. The inherent plasmonic characteristics of developed 2D nanojunction assembly accompanied by the commercial availability of acoustic activated technologies depict promising future for efficient and sustainable CO2 conversion in industrial levels.}},
articleno = {{119}},
author = {{Karbalaei Akbari, Mohammad and Lopa, Nasrin and Zhuiykov, Serge}},
booktitle = {{Proceedings of the 7th International Conference of Recent Trends in Environmental Science and Engineering (RTESE'23)}},
issn = {{2561-1089}},
keywords = {{CO2 Conversion,Two-Dimensional Materials,Plasmonic Photocatalysis,Nanotechnology and Environment}},
language = {{eng}},
location = {{Toronto, Canada}},
pages = {{5}},
title = {{Efficient and sustainable room-temperature CO2 conversion by plasmonic two-dimensional metal-oxide hybrid nano-interfaces}},
url = {{http://doi.org/10.11159/rtese23.119}},
year = {{2023}},
}
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